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The large resuspension of high molecular weight (HMW)-PAHs occurred, possibly related to frequent hydrodynamic disturbances. Furthermore, this study explored the distribution of PAHs among different compartments and the seasonal variation of multimedia transfers. Sensitivity analysis showed that the model is remarkably sensitive to four parameters including temperature and advection. Monte Carlo uncertainty analysis verified that the simulation results were stable and reliable. The results can provide a theoretical basis for the monitoring and control of shallow lake pollution.Nitrosamines, as a class of emerging frequently detected nitrogenous disinfection byproducts (N-DBPs) in drinking water, have gained increasing attention due to their potentially high health risk. Few studies focus on the occurrence variation and carcinogenic health risk of nitrosamines in drinking water systems. Our study aimed to investigate the spatial and temporal variability of nitrosamines in a drinking water system and to conduct a carcinogenic health risk assessment. Three types of water samples, including influent water, treated water and tap water, were collected monthly during an entire year in a drinking water system utilizing a combination of chlorine dioxide and chlorine in central China, and 9 nitrosamines were measured. The nitrosamine formation potentials (FPs) in influent water were also determined. N-nitrosodimethylamine (NDMA) was the most prevalent compound and was dominant in the water samples with average concentrations ranging from 2.5 to 67.4 ng/L, followed by N-nitrosodiethylamine (NDEA) and N-nitrosopiperidine (NPIP). Nitrosamine occurrence varied monthly, and significant seasonal differences were observed in tap water (p .05). The average and 95th percentile total lifetime cancer risks for the three main nitrosamines were 4.83 × 10-5 and 4.48 × 10-4, respectively, exceeding the negligible risk level (10-6) proposed by the USEPA. Exposure to nitrosamines in drinking water posed a higher cancer risk for children than for adults, and children aged 0.75 to 1 years suffered the highest cancer risk. These results suggest that nitrosamine occurrence in tap water varied temporally but not spatially. Exposure to drinking water nitrosamines may pose a carcinogenic risk to human health, especially to children.Arctic lakes emit methane (CH4) to the atmosphere. The magnitude of this flux could increase with permafrost thaw but might also be mitigated by microbial CH4 oxidation. Methane oxidation in oxic water has been extensively studied, while the contribution of anaerobic oxidation of methane (AOM) to CH4 mitigation is not fully understood. We have investigated four Northern Siberian stratified lakes in an area of discontinuous permafrost nearby Igarka, Russia. Analyses of CH4 concentrations in the water column demonstrated that 60 to 100% of upward diffusing CH4 was oxidized in the anoxic layers of the four lakes. A combination of pmoA and mcrA gene qPCR and 16S rRNA gene metabarcoding showed that the same taxa, all within Methylomonadaceae and including the predominant genus Methylobacter as well as Crenothrix, could be the major methane-oxidizing bacteria (MOB) in the anoxic water of the four lakes. Correlation between Methylomonadaceae and OTUs within Methylotenera, Geothrix and Geobacter genera indicated that AOM might occur in an interaction between MOB, denitrifiers and iron-cycling partners. We conclude that MOB within Methylomonadaceae could have a crucial impact on CH4 cycling in these Siberian Arctic lakes by mitigating the majority of produced CH4 before it leaves the anoxic zone. This finding emphasizes the importance of AOM by Methylomonadaceae and extends our knowledge about CH4 cycle in lakes, a crucial component of the global CH4 cycle.Aquatic plants are essential components in the regulation of microhabitat complexity and physico-chemical parameters in lake ecosystems. Increased eutrophication, land use change, modification of hydrological regimes, and expansion of invasive species are expected to impact aquatic plant community composition; however, historical pathways and response patterns are not well understood at the national scale. We analyzed temporal changes in aquatic plant communities in Japan from the early 1900s to the 2000s using field survey records from 248 lakes. Relationships of species associations with climate, land use, and lake characteristics were described using a joint species distribution model. The mean variation attributable to lake characteristics was 25.4%, followed by climate (14.0%), and land use (10.5%). Among the 13 functional traits used in our analysis, sexual and pollination traits showed marked responses to precipitation and land use. Hypohydrophily increased with precipitation, whereas monoecious aquatic plants increased in lakes surrounded by urbanized area. The relative ratio of floating to submerged plants has increased over time. Our results provide insight into long-term changes in aquatic plant communities and identify functional traits sensitive to environmental change.Compared with interdecadal, interannual, or seasonal scales, the variations of diurnal temperature range (DTR) at the intraseasonal scale and their driving forces are less understood. https://www.selleckchem.com/products/envonalkib.html Using surface meteorological observations and multi-source satellite retrievals during 2013-2017, together with Random Forest modeling, this study examines the intraseasonal variation of summer DTR in the Yangtze River Delta (YRD) region, China, and determines its potential driving factors [i.e., daily maximum/minimum surface air temperature (SATmax/SATmin), sunshine duration (SSD), rainfall, altitude, land vegetation cover, and land surface thermal environment including daytime/nighttime land surface temperature (LSTD/LSTN) and anthropogenic heat flux (AHF)]. It is found that the intraseasonal variation of DTR at both 8-day and monthly scales in the YRD exhibits regional differences and is modulated by different primary factors across the region. The evident intraseasonal variation of DTR, with a peak in June, in the northern Yhat experience various external forcings.
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