https://www.selleckchem.com/products/LDE225(NVP-LDE225).html In this paper, we present a quantum stochastic model for spectroscopic lineshapes in the presence of a co-evolving and non-stationary background population of excitations. Starting from a field theory description for interacting bosonic excitons, we derive a reduced model whereby optical excitons are coupled to an incoherent background via scattering as mediated by their screened Coulomb coupling. The Heisenberg equations of motion for the optical excitons are then driven by an auxiliary stochastic population variable, which we take to be the solution of an Ornstein-Uhlenbeck process. Itô's lemma then allows us to easily construct and evaluate correlation functions and response functions. Focusing on the linear response, we compare our model to the classic Anderson-Kubo model. While similar in motivation, there are differences in the predicted lineshapes, notably in terms of asymmetry, and variation with the increasing background population.Excited states of Coulomb systems are studied within density functional theory with information theoretical quantities. The Ghosh-Berkowitz-Parr thermodynamic transcription is extended to excited states, and the concept of the local temperature is introduced. It is shown that extremization of information entropy or Fisher information results in a constant temperature. For Coulomb systems, there is a simple relation between the total energy and phase-space Fisher information. The phase-space fidelity between excited states is proportional to the position-space fidelity, with a factor of proportionality depending on total energies. The phase-space relative entropy is equal to the position-space relative entropy plus a term depending only on the total energies. The relationship between the phase-space fidelity susceptibility and Fisher information is also presented.A first principles quantum formalism to describe the non-adiabatic dynamics of electrons and nuclei based on