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Advance applications like water splitting system and rechargeable metal-air battery are highly dependent on efficient electrocatalyst for the oxygen evolution reaction (OER). Heterostructured materials, with a high active surface area and electron effect, accomplish enhanced catalytic performance. Here, a nitride-sulfide composite (FeNi3N-Ni3S2) has been prepared by a simple hydrothermal process coupled with nitridation. The prepared composite electrocatalyst FeNi3N-Ni3S2 possesses lower electron densities compared to those of FeNi3N and Ni3S2, lessening the activation energy (Ea) toward the OER. Consequently, the prepared FeNi3N-Ni3S2 exhibits excellent OER performance with a low overpotential (230 mV) and a small Tafel slope (38 mV dec-1). Highly stable FeNi3N-Ni3S2 composite delivers lower charging voltage and extended lifetime in rechargeable Zn-air battery, compared with IrO2.As pure lubricants, ILs performed very well by forming the classical self-assembly bilayer at the sliding interface. The interface mechanism is still not clear in a very polar, e.g., water-based lubricating system. In this work, the interfacial absorption and tribological behavior of carboxylic alkanolamine ionic liquids (CAILs) serving as aqueous lubricating additives were studied by applying positive and negative potentials on the friction pair, accompanied by the comprehensive discussion of data from critical micelle concentration, quartz crystal microbalance, ECR, and MD results. The results reveal that the adsorption behavior, unexpectedly, was affected by the high polarity of H2O, where a less dense double-layer structure is observed at the interface by model imitation. Conversely, the monomolecular adsorption layer constructed electrostatically between the polar head (-COO-) and the positive base dominates the tribofilm. Meanwhile, the cations are partially accumulating around anions in the presence of static electricity, which does not form a neat and dense one-to-one corresponding cation-anion pair. In the solution, the IL maintains a state of dissociation and minor agglomeration. Furthermore, an increase in alkyl chains contributes to the thickness of the protective film generated by CAILs on the sliding asperity. Eventually, the synergistic effect from physical adsorption and the tribochemical reaction is responsible for excellent lubricity and antiwear performance of CAILs.Phosphoric acid (PA)-doped polybenzimidazoles generally require high PA doping levels to achieve high conductivity as high-temperature proton exchange membranes. However, high PA doping levels result in a significant decrease in the mechanical properties of and PA leaching from the membranes. Herein, a Zr-based metal-organic framework material (UIO-66) was introduced into poly[2,2'-(p-oxydiphenylene)-5,5'-benzimidazole] (OPBI) membranes. The composite membranes exhibited long-range continuous proton transport channels when the mass ratio of UIO-66 to OPBI was ≥30 wt %. The long-range continuous proton transport channels endowed the composite membranes with high proton conductivity at low PA doping levels. When the doping of UIO-66 in the OPBI membrane reached 40 wt %, the membrane exhibited the highest proton conductivity (0.092 S cm-1, at 160 °C) at a low PA uptake (73.25%), while the conductivity of the pristine OPBI membrane was 0.050 S cm-1 with a high PA uptake (217.43%). Additionally, in the oxyhydrogen fuel cell test, 40%UIO-66@OPBI membranes exhibited excellent fuel cell performance with a peak power density of 583 mW cm-2 at 160 °C, which is 50% higher than that of the pristine OPBI membrane (374 mW cm-2). A single cell based on 40%UIO-66@OPBI also demonstrated good durability and could remain at about 600 mV after 500 h of operation under a constant load of 200 mA cm-2.The following article has been retracted at the request of the authors, who performed a posteriori analysis of the data and identified inconsistencies that changed their evaluation of the results Barbalho M, Coswig VS, Steele J, Fisher JP, Giessing J, Gentil P. Evidence of a ceiling effect for training volume in muscle hypertrophy and strength in trained men-less is more? Int J Sports Physiol Perform. 2020;15(2)268-277. https://www.selleckchem.com/products/cdk2-inhibitor-73.html doi10.1123/ijspp.2018-0914. Hydrogen gas (H2) inhalation during hemorrhage stabilizes post-resuscitation hemodynamics, improving short-term survival in a rat hemorrhagic shock and resuscitation (HS/R) model. However, the underlying molecular mechanism of H2 in HS/R is unclear. Endothelial glycocalyx (EG) damage causes hemodynamic failure associated with HS/R. In this study, we tested the hypothesis that H2 alleviates oxidative stress by suppressing xanthine oxidoreductase (XOR) and/or preventing tumor necrosis factor-alfa (TNF-α)-mediated syndecan-1 shedding during EG damage. HS/R was induced in rats by reducing mean arterial pressure (MAP) to 35 mm Hg for 60 min followed by resuscitation. Rats inhaled oxygen or H2 + oxygen after achieving shock either in the presence or absence of an XOR inhibitor (XOR-I) for both the groups. In a second test, rats received oxygen alone or antitumor necrosis factor (TNF)-α monoclonal antibody with oxygen or H2. Two hours after resuscitation, XOR activity, purine metabolites, cytokines, syndecan-1 were measured and survival rates were assessed 6 h after resuscitation. H2 and XOR-I both suppressed MAP reduction and improved survival rates. H2 did not affect XOR activity and the therapeutic effects of XOR-I and H2 were additive. H2 suppressed plasma TNF-α and syndecan-1 expression; however, no additional H2 therapeutic effect was observed in the presence of anti-TNF-α monoclonal antibody. H2 inhalation after shock stabilized hemodynamics and improved survival rates in an HS/R model independent of XOR. The therapeutic action of H2 was partially mediated by inhibition of TNF-α-dependent syndecan-1 shedding. H2 inhalation after shock stabilized hemodynamics and improved survival rates in an HS/R model independent of XOR. The therapeutic action of H2 was partially mediated by inhibition of TNF-α-dependent syndecan-1 shedding.In a community-based birth cohort of 158 Australian infants followed to age 2 years, the incidence rate of human parainfluenza virus (HPIV) was 0.42 (95% CI = 0.33, 0.54) episodes per child-year with episodes occurring year-round, peaking in the spring season. HPIV-3 was the dominant subtype. Overall, 41% of detections were asymptomatic; only 32% of HPIV episodes led to healthcare contact with 1 hospitalization.
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